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Aratono, Yasuyuki; Wada, Akira*; Akiyama, Kazuhiko; Kitazawa, Shinichi; Hojo, Kiichi; Naramoto, Hiroshi*
Chemical Physics Letters, 408(4-6), p.247 - 251, 2005/06
Times Cited Count:1 Percentile:2.99(Chemistry, Physical)C fulleren was detected in the deposit produced by the laser ablation in superfluid helium at 1.5K. From the mass spectrometry, it was found that the ratio, C/CC, differs from statistical one calculated by Poisson distribution for natural graphite. Assuming the recombination of atomic carbons to C molecules as an initial stage for C formation, the different isotopic ratio of C from Poisson statistics was ascribed to the tunneling recombination between C and C atoms in the bubble state.